Fernando Pastawski, Norman Y. Yao, Liang Jiang, Mikhail D. Lukin, J. Ignacio Cirac
Dec 22, 2011·quant-ph·PDF The realization of devices which harness the laws of quantum mechanics represents an exciting challenge at the interface of modern technology and fundamental science. An exemplary paragon of the power of such quantum primitives is the concept of "quantum money". A dishonest holder of a quantum bank-note will invariably fail in any forging attempts; indeed, under assumptions of ideal measurements and decoherence-free memories such security is guaranteed by the no-cloning theorem. In any practical situation, however, noise, decoherence and operational imperfections abound. Thus, the development of secure "quantum money"-type primitives capable of tolerating realistic infidelities is of both practical and fundamental importance. Here, we propose a novel class of such protocols and demonstrate their tolerance to noise; moreover, we prove their rigorous security by determining tight fidelity thresholds. Our proposed protocols require only the ability to prepare, store and measure single qubit quantum memories, making their experimental realization accessible with current technologies.
Sungkun Hong, Michael S. Grinolds, Patrick Maletinsky, Ronald L. Walsworth, Mikhail D. Lukin, Amir Yacoby
The ability to control and manipulate spins via electrical, magnetic and optical means has generated numerous applications in metrology and quantum information science in recent years. A promising alternative method for spin manipulation is the use of mechanical motion, where the oscillation of a mechanical resonator can be magnetically coupled to a spins magnetic dipole, which could enable scalable quantum information architectures9 and sensitive nanoscale magnetometry. To date, however, only population control of spins has been realized via classical motion of a mechanical resonator. Here, we demonstrate coherent mechanical control of an individual spin under ambient conditions using the driven motion of a mechanical resonator that is magnetically coupled to the electronic spin of a single nitrogen-vacancy (NV) color center in diamond. Coherent control of this hybrid mechanical/spin system is achieved by synchronizing pulsed spin-addressing protocols (involving optical and radiofrequency fields) to the motion of the driven oscillator, which allows coherent mechanical manipulation of both the population and phase of the spin via motion-induced Zeeman shifts of the NV spins energy. We demonstrate applications of this coherent mechanical spin-control technique to sensitive nanoscale scanning magnetometry.
Dirk Englund, Brendan Shields, Kelley Rivoire, Fariba Hatami, Jelena Vuckovic, Hongkun Park, Mikhail D. Lukin
May 12, 2010·quant-ph·PDF We describe and experimentally demonstrate a technique for deterministic coupling between a photonic crystal (PC) nanocavity and single emitters. The technique is based on in-situ scanning of a PC cavity over a sample and allows the positioning of the cavity over a desired emitter with nanoscale resolution. The power of the technique, which we term a Scanning Cavity Microscope (SCM), is demonstrated by coupling the PC nanocavity to a single nitrogen vacancy (NV) center in diamond, an emitter system that provides optically accessible electron and nuclear spin qubits.
Norman Y. Yao, Liang Jiang, Alexey V. Gorshkov, Zhe-Xuan Gong, Alex Zhai, L. -M. Duan, Mikhail D. Lukin
Nov 11, 2010·quant-ph·PDF We propose and analyze a new approach for quantum state transfer between remote spin qubits. Specifically, we demonstrate that coherent quantum coupling between remote qubits can be achieved via certain classes of random, unpolarized (infinite temperature) spin chains. Our method is robust to coupling strength disorder and does not require manipulation or control over individual spins. In principle, it can be used to attain perfect state transfer over arbitrarily long range via purely Hamiltonian evolution and may be particularly applicable in a solid-state quantum information processor. As an example, we demonstrate that it can be used to attain strong coherent coupling between Nitrogen-Vacancy centers separated by micrometer distances at room temperature. Realistic imperfections and decoherence effects are analyzed.
Leigh S. Martin, Hengyun Zhou, Nathaniel T. Leitao, Nishad Maskara, Oksana Makarova, Haoyang Gao, Qian-Ze Zhu, Mincheol Park, Matthew Tyler, Hongkun Park, Soonwon Choi, Mikhail D. Lukin
Sep 19, 2022·quant-ph·PDF Understanding the microscopic mechanisms of thermalization in closed quantum systems is among the key challenges in modern quantum many-body physics. We demonstrate a method to probe local thermalization in a large-scale many-body system by exploiting its inherent disorder, and use this to uncover the thermalization mechanisms in a three-dimensional, dipolar-interacting spin system with tunable interactions. Utilizing advanced Hamiltonian engineering techniques to explore a range of spin Hamiltonians, we observe a striking change in the characteristic shape and timescale of local correlation decay as we vary the engineered exchange anisotropy. We show that these observations originate from the system's intrinsic many-body dynamics and reveal the signatures of conservation laws within localized clusters of spins, which do not readily manifest using global probes. Our method provides an exquisite lens into the tunable nature of local thermalization dynamics, and enables detailed studies of scrambling, thermalization and hydrodynamics in strongly-interacting quantum systems.
Alexey V. Gorshkov, Johannes Otterbach, Michael Fleischhauer, Thomas Pohl, Mikhail D. Lukin
Mar 18, 2011·quant-ph·PDF We develop the theory of light propagation under the conditions of electromagnetically induced transparency (EIT) in systems involving strongly interacting Rydberg states. Taking into account the quantum nature and the spatial propagation of light, we analyze interactions involving few-photon pulses. We demonstrate that this system can be used for the generation of nonclassical states of light including trains of single photons with an avoided volume between them, for implementing photon-photon quantum gates, as well as for studying many-body phenomena with strongly correlated photons.
Kartiek Agarwal, Ivar Martin, Mikhail D. Lukin, Eugene Demler
While two levels systems (TLSs) are ubiqitous in solid state systems, microscopic understanding of their nature remains an outstanding problem. Conflicting phenomenological models are used to describe TLSs in seemingly similar materials when probed with different experimental techniques. Specifically, bulk measurements in amorphous solids have been interpreted using the model of a tunneling atom or group of atoms, whereas TLSs observed in the insulating barriers of Josephson junction qubits have been understood in terms of tunneling of individual electrons. Motivated by recent experiments studying TLSs in Josephson junctions, especially the effects of elastic strain on TLS properties, we analyze interaction of the electronic TLS with phonons. We demonstrate that strong polaronic effects lead to dramatic changes in TLS properties. Our model gives a quantitative understanding of the TLS relaxation and dephasing as probed in Josephson junction qubits, while providing an alternative interpretation of bulk experiments. We demonstrate that a model of polaron dressed electronic TLS leads to estimates for the density and distribution of parameters of TLSs consistent with bulk experiments in amorphous solids. This model explains such surprising observations of recent experiments as the existence of minima in the energy of some TLSs as a function of strain and makes concrete predictions for the character of TLS dephasing near such minima. We argue that better understanding of the microscopic nature of TLSs can be used to improve properties of quantum devices, from an enhancement of relaxation time of TLSs, to creating new types of strongly interacting optomechanical systems.
Birgit J. M. Hausmann, Brendan Shields, Qimin Quan, Patrick Maletinsky, Murray McCutcheon, Jennifer T. Choy, Tom M. Babinec, Alexander Kubanek, Amir Yacoby, Mikhail D. Lukin, Marko Loncar
Nov 22, 2011·quant-ph·PDF Diamond is a unique material with exceptional physical and chemical properties that offers potential for the realization of high-performance devices with novel functionalities. For example diamond's high refractive index, transparency over wide wavelength range, and large Raman gain are of interest for the implementation of novel photonic devices. Recently, atom-like impurities in diamond emerged as an exceptional system for quantum information processing, quantum sensing and quantum networks. For these and other applications, it is essential to develop an integrated nanophotonic platform based on diamond. Here, we report on the realization of such an integrated diamond photonic platform, diamond on insulator (DOI), consisting of a thin single crystal diamond film on top of an insulating silicon dioxide/silicon substrate. Using this approach, we demonstrate diamond ring resonators that operate in a wide wavelength range, including the visible (630nm) and near-infrared (1,550nm). Finally, we demonstrate an integrated, on-chip quantum nanophotonic network, consisting of ring resonators coupled to low loss waveguides with grating couplers, that enables the generation and efficient routing of single photons at room temperature.
Rahul Sahay, Mikhail D. Lukin, Jordan Cotler
Jan 24, 2024·quant-ph·PDF The AdS/CFT correspondence stipulates a duality between conformal field theories and certain theories of quantum gravity in one higher spatial dimension. However, probing this conjecture on contemporary classical or quantum computers is challenging. We formulate an efficiently implementable multi-scale entanglement renormalization ansatz (MERA) model of AdS/CFT providing a mapping between a (1+1)-dimensional critical spin system and a (2+1)-dimensional bulk theory. Using a combination of numerics and analytics, we show that the bulk theory arising from this optimized tensor network furnishes excitations with attractive interactions. Remarkably, these excitations have one- and two-particle energies matching the predictions for matter coupled to AdS gravity at long distances, thus displaying key features of AdS physics. We show that these potentials arise as a direct consequence of entanglement renormalization and discuss how this approach can be used to efficiently simulate bulk dynamics using realistic quantum devices.
Murray W. McCutcheon, Darrick E. Chang, Yinan Zhang, Mikhail D. Lukin, Marko Loncar
Mar 26, 2009·quant-ph·PDF Motivated by developments in quantum information science, much recent effort has been directed toward coupling individual quantum emitters to optical microcavities. Such systems can be used to produce single photons on demand, enable nonlinear optical switching at a single photon level, and implement functional nodes of a quantum network, where the emitters serve as processing nodes and photons are used for long-distance quantum communication. For many of these practical applications, it is important to develop techniques that allow one to generate outgoing single photons of desired frequency and bandwidth, enabling hybrid networks connecting different types of emitters and long-distance transmission over telecommunications wavelengths. Here, we propose a novel approach that makes use of a nonlinear optical resonator, in which the single photon originating from the atom-like emitter is directly converted into a photon with desired frequency and bandwidth using the intracavity nonlinearity. As specific examples, we discuss a high-finesse, TE-TM double-mode photonic crystal cavity design that allows for direct generation of single photons at telecom wavelengths starting from an InAs/GaAs quantum dot with a 950 nm transition wavelength, and a scheme for direct optical coupling of such a quantum dot with a diamond nitrogen-vacancy center at 637 nm.
Paola Cappellaro, Mikhail D. Lukin
Apr 17, 2009·quant-ph·PDF We propose a strategy to generate a many-body entangled state in a collection of randomly placed, dipolarly coupled electronic spins in the solid state. By using coherent control to restrict the evolution into a suitable collective subspace, this method enables the preparation of GHZ-like and spin-squeezed states even for randomly positioned spins, while in addition protecting the entangled states against decoherence. We consider the application of this squeezing method to improve the sensitivity of nanoscale magnetometer based on Nitrogen-Vacancy spin qubits in diamond.
Michael Knap, Adrian Kantian, Thierry Giamarchi, Immanuel Bloch, Mikhail D. Lukin, Eugene Demler
We propose to use Ramsey interferometry and single-site addressability, available in synthetic matter such as cold atoms or trapped ions, to measure real-space and time resolved spin correlation functions. These correlation functions directly probe the excitations of the system, which makes it possible to characterize the underlying many-body states. Moreover they contain valuable information about phase transitions where they exhibit scale invariance. We also discuss experimental imperfections and show that a spin-echo protocol can be used to cancel slow fluctuations in the magnetic field. We explicitly consider examples of the two-dimensional, antiferromagnetic Heisenberg model and the one-dimensional, long-range transverse field Ising model to illustrate the technique.
Ashok Ajoy, Ulf Bissbort, Mikhail D. Lukin, Ronald L. Walsworth, Paola Cappellaro
Jul 11, 2014·quant-ph·PDF Nuclear spin imaging at the atomic level is essential for the understanding of fundamental biological phenomena and for applications such as drug discovery. The advent of novel nano-scale sensors has given hope of achieving the long-standing goal of single-protein, high spatial-resolution structure determination in their natural environment and ambient conditions. In particular, quantum sensors based on the spin-dependent photoluminescence of Nitrogen Vacancy (NV) centers in diamond have recently been used to detect nanoscale ensembles of external nuclear spins. While NV sensitivity is approaching single-spin levels, extracting relevant information from a very complex structure is a further challenge, since it requires not only the ability to sense the magnetic field of an isolated nuclear spin, but also to achieve atomic-scale spatial resolution. Here we propose a method that, by exploiting the coupling of the NV center to an intrinsic quantum memory associated with the Nitrogen nuclear spin, can reach a tenfold improvement in spatial resolution, down to atomic scales. The spatial resolution enhancement is achieved through coherent control of the sensor spin, which creates a dynamic frequency filter selecting only a few nuclear spins at a time. We propose and analyze a protocol that would allow not only sensing individual spins in a complex biomolecule, but also unraveling couplings among them, thus elucidating local characteristics of the molecule structure.
Dominik B. Bucher, David R. Glenn, Hongkun Park, Mikhail D. Lukin, Ronald L. Walsworth
Nuclear magnetic resonance (NMR) spectroscopy is a widely used tool for chemical analysis and molecular structure identification. Because it typically relies on the weak magnetic fields produced by a small thermal nuclear spin polarization, NMR suffers from poor molecule-number sensitivity compared to other analytical techniques. Recently, a new class of NMR sensors based on optically-probed nitrogen-vacancy (NV) quantum defects in diamond have allowed molecular spectroscopy from sample volumes several orders of magnitude smaller than the most sensitive inductive detectors. To date, however, NV-NMR spectrometers have only been able to observe signals from pure, highly concentrated samples. To overcome this limitation, we introduce a technique that combines picoliter-scale NV-NMR with fully integrated Overhauser dynamic nuclear polarization (DNP) to perform high-resolution spectroscopy on a variety of small molecules in dilute solution, with femtomole sensitivity. Our technique advances mass-limited NMR spectroscopy for drug and natural product discovery, catalysis research, and single cell studies.
Sorawis Sangtawesin, Bo L. Dwyer, Srikanth Srinivasan, James J. Allred, Lila V. H. Rodgers, Kristiaan De Greve, Alastair Stacey, Nikolai Dontschuk, Kane M. O'Donnell, Di Hu, D. Andrew Evans, Cherno Jaye, Daniel A. Fischer, Matthew L. Markham, Daniel J. Twitchen, Hongkun Park, Mikhail D. Lukin, Nathalie P. de Leon
The nitrogen vacancy (NV) center in diamond exhibits spin-dependent fluorescence and long spin coherence times under ambient conditions, enabling applications in quantum information processing and sensing. NV centers near the surface can have strong interactions with external materials and spins, enabling new forms of nanoscale spectroscopy. However, NV spin coherence degrades within 100 nanometers of the surface, suggesting that diamond surfaces are plagued with ubiquitous defects. Prior work on characterizing near-surface noise has primarily relied on using NV centers themselves as probes; while this has the advantage of exquisite sensitivity, it provides only indirect information about the origin of the noise. Here we demonstrate that surface spectroscopy methods and single spin measurements can be used as complementary diagnostics to understand sources of noise. We find that surface morphology is crucial for realizing reproducible chemical termination, and use these insights to achieve a highly ordered, oxygen-terminated surface with suppressed noise. We observe NV centers within 10 nm of the surface with coherence times extended by an order of magnitude.
Polnop Samutpraphoot, Tamara Ðorđević, Paloma L. Ocola, Hannes Bernien, Crystal Senko, Vladan Vuletić, Mikhail D. Lukin
Sep 19, 2019·quant-ph·PDF We demonstrate photon-mediated interactions between two individually trapped atoms coupled to a nanophotonic cavity. Specifically, we observe superradiant line broadening when the atoms are resonant with the cavity, and level repulsion when the cavity is coupled to the atoms in the dispersive regime. Our approach makes use of individual control over the internal states of the atoms, their position with respect to the cavity mode, as well as the light shifts to tune atomic transitions individually, allowing us to directly observe the anti-crossing of the superradiant and subradiant two-atom states. These observations open the door for realizing quantum networks and studying quantum many-body physics based on atom arrays coupled to nanophotonic devices.
Sambuddha Chattopadhyay, Hannes Pichler, Mikhail D. Lukin, Wen Wei Ho
Oct 17, 2019·quant-ph·PDF We study weak ergodicity breaking in a one-dimensional, nonintegrable spin-1 XY model. We construct for it an exact, highly excited eigenstate, which despite its large energy density, can be represented analytically by a finite bond-dimension matrix product state (MPS) with area-law entanglement. Upon a quench to a finite Zeeman field, the state undergoes periodic dynamics with perfect many-body revivals, in stark contrast to other generic initial states which instead rapidly thermalize. This dynamics can be completely understood in terms of the evolution of entangled virtual spin-1/2 degrees of freedom, which in turn underpin the presence of an extensive tower of strong-eigenstate thermalization hypothesis (ETH)-violating many-body eigenstates. The resulting quantum many-body scars are therefore of novel origin. Our results provide important analytical insights into the nature and entanglement structure of quantum many-body scars.
Luis A. Jauregui, Andrew Y. Joe, Kateryna Pistunova, Dominik S. Wild, Alexander A. High, You Zhou, Giovanni Scuri, Kristiaan De Greve, Andrey Sushko, Che-Hang Yu, Takashi Taniguchi, Kenji Watanabe, Daniel J. Needleman, Mikhail D. Lukin, Hongkun Park, Philip Kim
Excitons in semiconductors, bound pairs of excited electrons and holes, can form the basis for new classes of quantum optoelectronic devices. A van der Waals heterostructure built from atomically thin semiconducting transition metal dichalcogenides (TMDs) enables the formation of excitons from electrons and holes in distinct layers, producing interlayer excitons with large binding energy and a long lifetime. Employing heterostructures of monolayer TMDs, we realize optical and electrical generation of long-lived neutral and charged interlayer excitons. We demonstrate the transport of neutral interlayer excitons across the whole sample that can be controlled by excitation power and gate electrodes. We also realize the drift motion of charged interlayer excitons using Ohmic-contacted devices. The electrical generation and control of excitons provides a new route for realizing quantum manipulation of bosonic composite particles with complete electrical tunability.
Rivka Bekenstein, Igor Pikovski, Hannes Pichler, Ephraim Shahmoon, Susanne F. Yelin, Mikhail D. Lukin
Apr 15, 2019·quant-ph·PDF Metasurfaces mold the flow of classical light waves by engineering sub-wavelength patterns from dielectric or metallic thin films. We describe and analyze a method in which quantum operator-valued reflectivity can be used to control both spatio-temporal and quantum properties of transmitted and reflected light. Such a quantum metasurface is realized by preparing and manipulating entangled superposition states of atomically thin reflectors. Specifically, we show that such a system allows for massively parallel quantum operations between atoms and photons and for the generation of highly non-classical states of light, including photonic GHZ and cluster states suitable for quantum information processing. We analyze the influence of imperfections and decoherence, as well as specific implementations based on atom arrays excited into Rydberg states. Finally, the extension to quantum metamaterials and emulations of quantum gravitational background for light are discussed.
Hengyun Zhou, Joonhee Choi, Soonwon Choi, Renate Landig, Alexander M. Douglas, Junichi Isoya, Fedor Jelezko, Shinobu Onoda, Hitoshi Sumiya, Paola Cappellaro, Helena S. Knowles, Hongkun Park, Mikhail D. Lukin
Jul 23, 2019·quant-ph·PDF Quantum metrology makes use of coherent superpositions to detect weak signals. While in principle the sensitivity can be improved by increasing the density of sensing particles, in practice this improvement is severely hindered by interactions between them. Using a dense ensemble of interacting electronic spins in diamond, we demonstrate a novel approach to quantum metrology. It is based on a new method of robust quantum control, which allows us to simultaneously eliminate the undesired effects associated with spin-spin interactions, disorder and control imperfections, enabling a five-fold enhancement in coherence time compared to conventional control sequences. Combined with optimal initialization and readout protocols, this allows us to break the limit for AC magnetic field sensing imposed by interactions, opening a promising avenue for the development of solid-state ensemble magnetometers with unprecedented sensitivity.