Cornelis Jacobus van Diepen, Vasiliki Angelopoulou, Oliver August Dall'Alba Sandberg, Alexey Tiranov, Ying Wang, Sven Scholz, Arne Ludwig, Anders Søndberg Sørensen, Peter Lodahl
Feb 24, 2025·quant-ph·PDF Waveguide quantum electrodynamics (QED) has opened a new frontier in quantum optics, which enables the radiative coupling of distantly located emitters via the spatially extended waveguide mode. This coupling leads to modified emission dynamics and previous work has reported the observation of increased intensity correlations (an antidip) when probing the resonance response of multiple emitters. However, the interference between independent emitters has been shown to lead to a similar response. Here, we directly observe resonant energy transfer between two distant quantum emitters by recording an antidip in the intensity correlations, $g^{(2)}(τ)$, while driving only one of the emitters. Under the condition that only a single emitter is driven, the antidip in photon coincidences is a distinctive signature of emitter-emitter coupling, which enables the transfer of energy from the driven to the undriven emitter. Interestingly, the observed mechanism is a long-range and waveguide-engineered version of resonant Förster transfer, which is responsible for the transport of energy between chlorophylls in the photosynthesis. Building on the established coupling, we demonstrate collective driving of the coupled emitter pair. Specifically, we control the relative driving phase and amplitude of the emitters and apply this collective excitation scheme to selectively populate the long-lived subradiant state. This results in suppressed emission, i.e. the peculiar situation where driving two emitters as opposed to one effectively reduces the probability of photon emission. Our work presents novel emission regimes and excitation schemes for a multi-emitter waveguide QED system. These can be exploited to deterministically generate emitter-emitter entanglement and advanced photonic states providing robustness against losses for photonic quantum computation and quantum communication.
Alexey Tiranov, Vasiliki Angelopoulou, Cornelis Jacobus van Diepen, Björn Schrinski, Oliver August Dall'Alba Sandberg, Ying Wang, Leonardo Midolo, Sven Scholz, Andreas Dirk Wieck, Arne Ludwig, Anders Søndberg Sørensen, Peter Lodahl
Photon emission is the hallmark of light-matter interaction and the foundation of photonic quantum science, enabling advanced sources for quantum communication and computing. Although single-emitter radiation can be tailored by the photonic environment, the introduction of multiple emitters extends this picture. A fundamental challenge, however, is that the radiative dipole-dipole coupling rapidly decays with spatial separation, typically within a fraction of the optical wavelength. We realize distant dipole-dipole radiative coupling with pairs of solid-state optical quantum emitters embedded in a nanophotonic waveguide. We dynamically probe the collective response and identify both super- and subradiant emission as well as means to control the dynamics by proper excitation techniques. Our work constitutes a foundational step toward multiemitter applications for scalable quantum-information processing.
Adrien Signoles, Baptiste Lecoutre, Jérémie Richard, Lih-King Lim, Vincent Denechaud, Valentin V. Volchkov, Vasiliki Angelopoulou, Fred Jendrzejewski, Alain Aspect, Laurent Sanchez-Palencia, Vincent Josse
We study the elastic scattering time $τ_\mathrm{s}$ of ultracold atoms propagating in optical disordered potentials in the strong scattering regime, going beyond the recent work of J. Richard \emph{et al.} \textit{Phys. Rev. Lett.} \textbf{122} 100403 (2019). There, we identified the crossover between the weak and the strong scattering regimes by comparing direct measurements and numerical simulations to the first order Born approximation. Here we focus specifically on the strong scattering regime, where the first order Born approximation is not valid anymore and the scattering time is strongly influenced by the nature of the disorder. To interpret our observations, we connect the scattering time $τ_\mathrm{s}$ to the profiles of the spectral functions that we estimate using higher order Born perturbation theory or self-consistent Born approximation. The comparison reveals that self-consistent methods are well suited to describe $τ_\mathrm{s}$ for Gaussian-distributed disorder, but fails for laser speckle disorder. For the latter, we show that the peculiar profiles of the spectral functions, as measured independently in V. Volchkov \emph{et al.} \textit{Phys. Rev. Lett.} \textbf{120}, 060404 (2018), must be taken into account. Altogether our study characterizes the validity range of usual theoretical methods to predict the elastic scattering time of matter waves, which is essential for future close comparison between theory and experiments, for instance regarding the ongoing studies on Anderson localization.
Xiao-Liu Chu, Vasiliki Angelopoulou, Peter Lodahl, Nir Rotenberg
Coherent interactions between quantum emitters in tailored photonic structures is a fundamental building block for future quantum technologies, but remains challenging to observe in complex solid-state environments, where the role of decoherence must be considered. Here, we investigate the optical interaction between two quantum emitters mediated by one-dimensional waveguides in a realistic solid-state environment, focusing on the creation, population and detection of a sub-radiant state, in the presence of dephasing. We show that as dephasing increases, the signatures of sub-radiance quickly vanish in intensity measurements yet remain pronounced in photon correlation measurements, particularly when the two emitters are pumped separately so as to populate the sub-radiant state efficiently. The applied Green's tensor approach is used to model a photonic crystal waveguide, including the dependence on the spatial position of the integrated emitter. The work lays out a route to the experimental realization of sub-radiant states in nanophotonic waveguides containing solid-state emitters.
Clara Henke, Thomas Wilkens Sandø, Vasiliki Angelopoulou, Lena Maria Hansen, Alexey Tiranov, Oliver August Dall'Alba Sandberg, Zhe Liu, Leonardo Midolo, Nikolai Bart, Arne Ludwig, Anders Søndberg Sørensen, Peter Lodahl, Cornelis Jacobus van Diepen
Radiative coupling between quantum emitters leads to a range of spectacular emission phenomena. Dicke studied the foundations of collectively enhanced and suppressed decay, commonly referred to as super- and subradiance. Collective effects can further result in directionality of the emission, thus offering a complimentary implementation of chiral quantum optics. Waveguide quantum electrodynamics (QED) allows coupling between spatially separated emitters, enabling selective driving. In this work, we control the emission direction for a pair of quantum dots embedded in a bidirectional photonic crystal waveguide offering independent electrical tuning. Notably the emitters are 13 \micro m apart, which corresponds to 26 effective wavelengths, but are nevertheless radiatively coupled. The directionality arises from a dispersive dipole-dipole interaction, which shifts the energy of the collective states, so that the emitter pair effectively forms an artificial molecule. We show that the emission direction can be switched from left- to rightwards by manipulating the relative driving phase while collectively exciting the emitters. In addition, we observe directional photon statistics under continuous driving, with, for example, single photons detected on one output port, and photon pairs on the other. With pulsed excitation, both emitters are fully inverted and correlated photon pairs are observed in time-resolved intensity correlation measurements. This work demonstrates a novel implementation of chiral quantum optics using quantum dots coupled via a non-chiral waveguide, and reports key steps for scaling up as a multi-emitter waveguide QED platform.