Manuel Endres, Takeshi Fukuhara, David Pekker, Marc Cheneau, Peter Schauß, Christian Gross, Eugene Demler, Stefan Kuhr, Immanuel Bloch
Spontaneous symmetry breaking plays a key role in our understanding of nature. In a relativistic field theory, a broken continuous symmetry leads to the emergence of two types of fundamental excitations: massless Nambu-Goldstone modes and a massive `Higgs' amplitude mode. An excitation of Higgs type is of crucial importance in the standard model of elementary particles and also appears as a fundamental collective mode in quantum many-body systems. Whether such a mode exists in low-dimensional systems as a resonance-like feature or becomes over-damped through coupling to Nambu-Goldstone modes has been a subject of theoretical debate. Here we reveal and study a Higgs mode in a two-dimensional neutral superfluid close to the transition to a Mott insulating phase. We unambiguously identify the mode by observing the expected softening of the onset of spectral response when approaching the quantum critical point. In this regime, our system is described by an effective relativistic field theory with a two-component quantum-field, constituting a minimal model for spontaneous breaking of a continuous symmetry. Additionally, all microscopic parameters of our system are known from first principles and the resolution of our measurement allows us to detect excited states of the many-body system at the level of individual quasiparticles. This allows for an in-depth study of Higgs excitations, which also addresses the consequences of reduced dimensionality and confinement of the system. Our work constitutes a first step in exploring emergent relativistic models with ultracold atomic gases.
Lucia Hackermuller, Ulrich Schneider, Maria Moreno-Cardoner, Takuya Kitagawa, Sebastian Will, Thorsten Best, Eugene Demler, Ehud Altman, Immanuel Bloch, Belen Paredes
Strong correlations can dramatically modify the thermodynamics of a quantum many-particle system. Especially intriguing behaviour can appear when the system adiabatically enters a strongly correlated regime, for the interplay between entropy and strong interactions can lead to counterintuitive effects. A well known example is the so-called Pomeranchuk effect, occurring when liquid 3He is adiabatically compressed towards its crystalline phase. Here, we report on a novel anomalous, isentropic effect in a spin mixture of attractively interacting fermionic atoms in an optical lattice. As we adiabatically increase the attraction between the atoms we observe that the gas, instead of contracting, anomalously expands. This expansion results from the combination of two effects induced by pair formation in a lattice potential: the suppression of quantum fluctuations as the attraction increases, which leads to a dominant role of entropy, and the progressive loss of the spin degree of freedom, which forces the gas to excite additional orbital degrees of freedom and expand to outer regions of the trap in order to maintain the entropy. The unexpected thermodynamics we observe reveal fundamentally distinctive features of pairing in the fermionic Hubbard model.
Yu-Ao Chen, Sebastian D. Huber, Stefan Trotzky, Immanuel Bloch, Ehud Altman
The Landau-Zener model of a quantum mechanical two-level system driven with a linearly time dependent detuning has served over decades as a textbook paradigm of quantum dynamics. In their seminal work [L. D. Landau, Physik. Z. Sowjet. 2, 46 (1932); C. Zener, Proc. Royal Soc. London 137, 696 (1932)], Landau and Zener derived a non-perturbative prediction for the transition probability between two states, which often serves as a reference point for the analysis of more complex systems. A particularly intriguing question is whether that framework can be extended to describe many-body quantum dynamics. Here we report an experimental and theoretical study of a system of ultracold atoms, offering a direct many-body generalization of the Landau-Zener problem. In a system of pairwise tunnel-coupled 1D Bose liquids we show how tuning the correlations of the 1D gases, the tunnel coupling between the tubes and the inter-tube interactions strongly modify the original Landau-Zener picture. The results are explained using a mean-field description of the inter-tube condensate wave-function, coupled to the low-energy phonons of the 1D Bose liquid.
Xing-Yan Chen, Andreas Schindewolf, Sebastian Eppelt, Roman Bause, Marcel Duda, Shrestha Biswas, Tijs Karman, Timon Hilker, Immanuel Bloch, Xin-Yu Luo
Scattering resonances are an essential tool for controlling interactions of ultracold atoms and molecules. However, conventional Feshbach scattering resonances, which have been extensively studied in various platforms, are not expected to exist in most ultracold polar molecules due to the fast loss that occurs when two molecules approach at a close distance. Here, we demonstrate a new type of scattering resonances that is universal for a wide range of polar molecules. The so-called field-linked resonances occur in the scattering of microwave-dressed molecules due to stable macroscopic tetramer states in the intermolecular potential. We identify two resonances between ultracold ground-state sodium-potassium molecules and use the microwave frequencies and polarizations to tune the inelastic collision rate by three orders of magnitude, from the unitary limit to well below the universal regime. The field-linked resonance provides a tuning knob to independently control the elastic contact interaction and the dipole-dipole interaction, which we observe as a modification in the thermalization rate. Our result provides a general strategy for resonant scattering between ultracold polar molecules, which paves the way for realizing dipolar superfluids and molecular supersolids as well as assembling ultracold polyatomic molecules.
Elisabeth Wybo, Alvise Bastianello, Monika Aidelsburger, Immanuel Bloch, Michael Knap
The sine-Gordon model emerges as a low-energy theory in a plethora of quantum many-body systems. Here, we theoretically investigate tunnel-coupled Bose-Hubbard chains with strong repulsive interactions as a realization of the sine-Gordon model deep in the quantum regime. We propose protocols for quantum gas microscopes of ultracold atoms to prepare and analyze solitons, that are the fundamental topological excitations of the emergent sine-Gordon theory. With numerical simulations based on matrix product states we characterize the preparation and detection protocols and discuss the experimental requirements.
Xing-Yan Chen, Marcel Duda, Andreas Schindewolf, Roman Bause, Immanuel Bloch, Xin-Yu Luo
We study three-body loss in an ultracold mixture of a thermal Bose gas and a degenerate Fermi gas. We find that at unitarity, where the interspecies scattering length diverges, the usual inverse-square temperature scaling of the three-body loss found in non-degenerate systems is strongly modified and reduced with the increasing degeneracy of the Fermi gas. While the reduction of loss is qualitatively explained within the few-body scattering framework, a remaining suppression provides evidence for the long-range RKKY interactions mediated by fermions between bosons. Our model based on RKKY interactions quantitatively reproduces the data without free parameters, and predicts one order of magnitude reduction of the three-body loss coefficient in the deeply Fermi-degenerate regime.
Martin Boll, Timon A. Hilker, Guillaume Salomon, Ahmed Omran, Jacopo Nespolo, Lode Pollet, Immanuel Bloch, Christian Gross
The repulsive Hubbard Hamiltonian is one of the foundational models describing strongly correlated electrons and is believed to capture essential aspects of high temperature superconductivity. Ultracold fermions in optical lattices allow for the simulation of the Hubbard Hamiltonian with a unique control over kinetic energy, interactions and doping. A great challenge is to reach the required low entropy and to observe antiferromagnetic spin correlations beyond nearest neighbors, for which quantum gas microscopes are ideal. Here we report on the direct, single-site resolved detection of antiferromagnetic correlations extending up to three sites in spin-$1/2$ Hubbard chains, which requires an entropy well below $s^*=\ln(2)$. Finally, the simultaneous detection of spin and density opens the route towards the study of the interplay between magnetic ordering and doping in various dimensions.
Pranjal Bordia, Henrik Lüschen, Ulrich Schneider, Michael Knap, Immanuel Bloch
We experimentally study a periodically driven many-body localized system realized by interacting fermions in a one-dimensional quasi-disordered optical lattice. By preparing the system in a far-from-equilibrium state and monitoring the remains of an imprinted density pattern, we identify a localized phase at high drive frequencies and an ergodic phase at low ones. These two distinct phases are separated by a dynamical phase transition which depends on both the drive frequency and the drive strength. Our observations are quantitatively supported by numerical simulations and are directly connected to the change in the statistical properties of the effective Floquet Hamiltonian.
Henrik P. Lüschen, Pranjal Bordia, Sebastian Scherg, Fabien Alet, Ehud Altman, Ulrich Schneider, Immanuel Bloch
In the presence of sufficiently strong disorder or quasiperiodic fields, an interacting many-body system can fail to thermalize and become many-body localized. The associated transition is of particular interest, since it occurs not only in the ground state but over an extended range of energy densities. So far, theoretical studies of the transition have focused mainly on the case of true-random disorder. In this work, we experimentally and numerically investigate the regime close to the many-body localization transition in quasiperiodic systems. We find slow relaxation of the density imbalance close to the transition, strikingly similar to the behavior near the transition in true-random systems. This dynamics is found to continuously slow down upon approaching the transition and allows for an estimate of the transition point. We discuss possible microscopic origins of these slow dynamics.
Simon Karch, Souvik Bandyopadhyay, Zheng-Hang Sun, Alexander Impertro, SeungJung Huh, Irene Prieto Rodríguez, Julian F. Wienand, Wolfgang Ketterle, Markus Heyl, Anatoli Polkovnikov, Immanuel Bloch, Monika Aidelsburger
The Loschmidt echo - the probability of a quantum many-body system to return to its initial state following a dynamical evolution - generally contains key information about a quantum system, relevant across various scientific fields including quantum chaos, quantum many-body physics, or high-energy physics. However, it is typically exponentially small in system size, posing an outstanding challenge for experiments. Here, we experimentally investigate the subsystem Loschmidt echo, a quasi-local observable that captures key features of the Loschmidt echo while being readily accessible experimentally. Utilizing quantum gas microscopy, we study its short- and long-time dynamics. In the short-time regime, we observe a dynamical quantum phase transition arising from genuine higher-order correlations. In the long-time regime, the subsystem Loschmidt echo allows us to quantitatively determine the effective dimension and structure of the accessible Hilbert space in the thermodynamic limit. Performing these measurements in the ergodic regime and in the presence of emergent kinetic constraints, we provide direct experimental evidence for ergodicity breaking due to fragmentation of the Hilbert space. Our results establish the subsystem Loschmidt echo as a novel and powerful tool that allows paradigmatic studies of both non-equilibrium dynamics and equilibrium thermodynamics of quantum many-body systems, applicable to a broad range of quantum simulation and computing platforms.
Shrestha Biswas, Sebastian Eppelt, Christian Buchberger, Xing-Yan Chen, Andreas Schindewolf, Michael Hani, Erwin Biebl, Immanuel Bloch, Xin-Yu Luo
Microwave(MW) fields with strong field strength, ultralow phase-noise and tunable polarization are crucial for stabilizing and manipulating ultracold polar molecules, which have emerged as a promising platform for quantum sciences. In this letter, we present the design, characterization, and performance of a robust MW setup tailored for precise control of molecular states. This setup achieves a high electric field intensity of 6.9 kV/m in the near-field from a dual-feed waveguide antenna, enabling a Rabi frequency as high as 71 MHz for the rotational transition of sodium-potassium molecules. In addition, the low noise signal source and controlled electronics provide ultralow phase-noise and dynamically tunable polarization. Narrow-band filters within the MW circuitry further reduce phase-noise by more than 20 dB at 20 MHz offset frequency, ensuring prolonged one-body molecular lifetimes up to 10 seconds. We also show practical methods to measure the MW field strength and polarization using a simple homemade dipole probe, and to characterize phase-noise down to -170 dBc/Hz with a commercial spectrum analyser and a notch filter. Those capabilities allowed us to evaporatively cool our molecular sample to deep quantum degeneracy. Furthermore, the polarization tunability enabled the observation of field-linked resonances and facilitated the creation of field-linked tetramers.These techniques advance the study of ultracold polar molecules and broaden the potential applications of MW tools in other platforms of quantum sciences.
Thomas Kohlert, Sebastian Scherg, Xiao Li, Henrik P. Lüschen, Sankar Das Sarma, Immanuel Bloch, Monika Aidelsburger
We experimentally study many-body localization (MBL) with ultracold atoms in a weak one-dimensional quasiperiodic potential, which in the noninteracting limit exhibits an intermediate phase that is characterized by a mobility edge. We measure the time evolution of an initial charge density wave after a quench and analyze the corresponding relaxation exponents. We find clear signatures of MBL, when the corresponding noninteracting model is deep in the localized phase. We also critically compare and contrast our results with those from a tight-binding Aubry-André model, which does not exhibit a single-particle intermediate phase, in order to identify signatures of a potential many-body intermediate phase.
Daniel Adler, David Wei, Melissa Will, Kritsana Srakaew, Suchita Agrawal, Pascal Weckesser, Roderich Moessner, Frank Pollmann, Immanuel Bloch, Johannes Zeiher
The relaxation behaviour of isolated quantum systems taken out of equilibrium is among the most intriguing questions in many-body physics. Quantum systems out of equilibrium typically relax to thermal equilibrium states by scrambling local information and building up entanglement entropy. However, kinetic constraints in the Hamiltonian can lead to a breakdown of this fundamental paradigm due to a fragmentation of the underlying Hilbert space into dynamically decoupled subsectors in which thermalisation can be strongly suppressed. Here, we experimentally observe Hilbert space fragmentation (HSF) in a two-dimensional tilted Bose-Hubbard model. Using quantum gas microscopy, we engineer a wide variety of initial states and find a rich set of manifestations of HSF involving bulk states, interfaces and defects, i.e., d = 2, 1 and 0 dimensional objects. Specifically, uniform initial states with equal particle number and energy differ strikingly in their relaxation dynamics. Inserting controlled defects on top of a global, non-thermalising chequerboard state, we observe highly anisotropic, sub-dimensional dynamics, an immediate signature of their fractonic nature. An interface between localized and thermalising states in turn displays dynamics depending on its orientation. Our results mark the first observation of HSF beyond one dimension, as well as the concomitant direct observation of fractons, and pave the way for in-depth studies of microscopic transport phenomena in constrained systems
David Wei, Daniel Adler, Kritsana Srakaew, Suchita Agrawal, Pascal Weckesser, Immanuel Bloch, Johannes Zeiher
The Mott-insulating phase of the two-dimensional (2d) Bose-Hubbard model is expected to be characterized by a non-local brane parity order. Parity order captures the presence of microscopic particle-hole fluctuations and entanglement, whose properties depend on the underlying lattice geometry. We realize 2d Bose-Hubbard models in dynamically tunable lattice geometries, using neutral atoms in a novel passively phase-stable tunable optical lattice in combination with programmable site-blocking potentials. We benchmark the performance of our system by single-particle quantum walks in the square, triangular, kagome and Lieb lattice. In the strongly correlated regime, we microscopically characterize the geometry dependence of the quantum fluctuations and experimentally validate the brane parity as a proxy for the non-local order parameter signaling the superfluid-to-Mott insulating phase transition.
Monika Aidelsburger, Marcos Atala, Sylvain Nascimbène, Stefan Trotzky, Yu-Ao Chen, Immanuel Bloch
We use Raman-assisted tunneling in an optical superlattice to generate large tunable effective magnetic fields for ultracold atoms. When hopping in the lattice, the accumulated phase shift by an atom is equivalent to the Aharonov-Bohm phase of a charged particle exposed to a staggered magnetic field of large magnitude, on the order of one flux quantum per plaquette. We study the ground state of this system and observe that the frustration induced by the magnetic field can lead to a degenerate ground state for non-interacting particles. We provide a measurement of the local phase acquired from Raman-induced tunneling, demonstrating time-reversal symmetry breaking of the underlying Hamiltonian. Furthermore, the quantum cyclotron orbit of single atoms in the lattice exposed to the magnetic field is directly revealed.
Antonio Rubio-Abadal, Matteo Ippoliti, Simon Hollerith, David Wei, Jun Rui, S. L. Sondhi, Vedika Khemani, Christian Gross, Immanuel Bloch
Periodic driving has emerged as a powerful tool in the quest to engineer new and exotic quantum phases. While driven many-body systems are generically expected to absorb energy indefinitely and reach an infinite-temperature state, the rate of heating can be exponentially suppressed when the drive frequency is large compared to the local energy scales of the system -- leading to long-lived 'prethermal' regimes. In this work, we experimentally study a bosonic cloud of ultracold atoms in a driven optical lattice and identify such a prethermal regime in the Bose-Hubbard model. By measuring the energy absorption of the cloud as the driving frequency is increased, we observe an exponential-in-frequency reduction of the heating rate persisting over more than 2 orders of magnitude. The tunability of the lattice potentials allows us to explore one- and two-dimensional systems in a range of different interacting regimes. Alongside the exponential decrease, the dependence of the heating rate on the frequency displays features characteristic of the phase diagram of the Bose-Hubbard model, whose understanding is additionally supported by numerical simulations in one dimension. Our results show experimental evidence of the phenomenon of Floquet prethermalization, and provide insight into the characterization of heating for driven bosonic systems.
Simon Hollerith, Johannes Zeiher, Jun Rui, Antonio Rubio-Abadal, Valentin Walther, Thomas Pohl, Dan M. Stamper-Kurn, Immanuel Bloch, Christian Gross
A microscopic understanding of molecules is essential for many fields of natural sciences but their tiny size hinders direct optical access to their constituents. Rydberg macrodimers - bound states of two highly-excited Rydberg atoms - feature bond lengths easily exceeding optical wavelengths. Here we report on the direct microscopic observation and detailed characterization of such macrodimers in a gas of ultracold atoms in an optical lattice. The size of about 0.7 micrometers, comparable to the size of small bacteria, matches the diagonal distance of the lattice. By exciting pairs in the initial two-dimensional atom array, we resolve more than 50 vibrational resonances. Using our spatially resolved detection, we observe the macrodimers by correlated atom loss and demonstrate control of the molecular alignment by the choice of the vibrational state. Our results allow for precision testing of Rydberg interaction potentials and establish quantum gas microscopy as a powerful new tool for quantum chemistry.
Simon Hollerith, Jun Rui, Antonio Rubio-Abadal, Kritsana Srakaew, David Wei, Johannes Zeiher, Christian Gross, Immanuel Bloch
Precise control and study of molecules is challenging due to the variety of internal degrees of freedom and local coordinates that are typically not controlled in an experiment. Employing quantum gas microscopy to position and resolve the atoms in Rydberg macrodimer states solves almost all of these challenges and enables unique access to the molecular frame. Here, we demonstrate the power of this approach and present first photoassociation studies for different molecular symmetries in which the molecular orientation relative to an applied magnetic field, the polarization of the excitation light and the initial atomic state are fully controlled. The observed characteristic dependencies allow for an electronic structure tomography of the molecular state. We additionally observe an orientation-dependent Zeeman shift and reveal a significant influence on it caused by the hyperfine interaction of the macrodimer state. Finally, we demonstrate controlled engineering of the electrostatic binding potential by opening a gap in the energetic vicinity of two crossing pair potentials.
Guillaume Salomon, Joannis Koepsell, Jayadev Vijayan, Timon A. Hilker, Jacopo Nespolo, Lode Pollet, Immanuel Bloch, Christian Gross
The interplay between magnetism and doping is at the origin of exotic strongly correlated electronic phases and can lead to novel forms of magnetic ordering. One example is the emergence of incommensurate spin-density waves with a wave vector that does not match the reciprocal lattice. In one dimension this effect is a hallmark of Luttinger liquid theory, which also describes the low energy physics of the Hubbard model. Here we use a quantum simulator based on ultracold fermions in an optical lattice to directly observe such incommensurate spin correlations in doped and spin-imbalanced Hubbard chains using fully spin and density resolved quantum gas microscopy. Doping is found to induce a linear change of the spin-density wave vector in excellent agreement with Luttinger theory predictions. For non-zero polarization we observe a decrease of the wave vector with magnetization as expected from the Heisenberg model in a magnetic field. We trace the microscopic origin of these incommensurate correlations to holes, doublons and excess spins which act as delocalized domain walls for the antiferromagnetic order. Finally, when inducing interchain coupling we observe fundamentally different spin correlations around doublons indicating the formation of a magnetic polaron.
Antonio Rubio-Abadal, Jae-yoon Choi, Johannes Zeiher, Simon Hollerith, Jun Rui, Immanuel Bloch, Christian Gross
Closed generic quantum many-body systems may fail to thermalize under certain conditions even after long times, a phenomenon called many-body localization (MBL). Numerous studies support the stability of the MBL phase in strongly disordered one-dimensional systems. However, the situation is much less clear when a small part of the system is ergodic, a scenario which also has important implications for the existence of many-body localization in higher dimensions. Here we address this question experimentally using a large-scale quantum simulator of ultracold bosons in a two-dimensional optical lattice. We prepare two-component mixtures of varying relative population and implement a disorder potential which is only experienced by one of the components. The second non-disordered ''clean'' component plays the role of a bath of adjustable size that is collisionally coupled to the ''dirty'' component. Our experiments show how the dynamics of the dirty component, which, when on its own, show strong evidence of localization, become affected by the coupling to the clean component. For a high clean population, the clean component appears to behave as an effective bath for the system which leads to its delocalization, while for a smaller clean population, the ability of the bath to destabilize the system becomes strongly reduced. Our results reveal how a finite-sized quantum system can bring another one towards thermalization, in a regime of complex interplay between disorder, tunneling and intercomponent interactions. They provide a new benchmark for effective theories aiming to capture the complex physics of MBL in the weakly localized regime.