David Neubauer, Artem V. Pronin, Sina Zapf, Johannes Merz, Hirale S. Jeevan, Wen-He Jiao, Philipp Gegenwart, Guang-Han Cao, Martin Dressel
We present a broadband optical-conductivity study of superconducting single-crystalline EuFe2(As1-xPx)2 with three different substitutional levels. We analyze the normal-state electrodynamics by decomposing the conductivity spectra using a Drude-Lorentz model with two Drude terms representing two groups of carriers with different scattering rates. The analysis reveals that the scattering rate of at least one of the Drude components develops linearly with temperature for each doping level. This points towards strong electron-electron correlations and a non-Fermi-liquid behavior in the P-substituted superconducting Eu-122 pnictides. We also detect a transfer of the spectral weight from mid-infrared to higher frequencies and assign it to the Hund's-rule coupling between itinerant and localized carriers. The conductivity spectra below the superconducting transition show no sharp features to be associated with the dirty-limit superconducting BCS gaps. We interpret these results in terms of clean-limit superconductivity in EuFe2(As1-xPx)2. The best parametrization fit can be achieved using a two-gap model. We find that the larger gap at the hole pockets of the Fermi surface is likely to be isotropic, while the smaller gap at the electron pockets is anisotropic or even nodal.
Kai Jeggle, Mikolaj Czerkawski, Federico Serva, Bertrand Le Saux, David Neubauer, Ulrike Lohmann
IceCloudNet is a novel method based on machine learning able to predict high-quality vertically resolved cloud ice water contents (IWC) and ice crystal number concentrations (N$_\textrm{ice}$). The predictions come at the spatio-temporal coverage and resolution of geostationary satellite observations (SEVIRI) and the vertical resolution of active satellite retrievals (DARDAR). IceCloudNet consists of a ConvNeXt-based U-Net and a 3D PatchGAN discriminator model and is trained by predicting DARDAR profiles from co-located SEVIRI images. Despite the sparse availability of DARDAR data due to its narrow overpass, IceCloudNet is able to predict cloud occurrence, spatial structure, and microphysical properties with high precision. The model has been applied to ten years of SEVIRI data, producing a dataset of vertically resolved IWC and N$_\textrm{ice}$ of clouds containing ice with a 3 kmx3 kmx240 mx15 minute resolution in a spatial domain of 30°W to 30°E and 30°S to 30°N. The produced dataset increases the availability of vertical cloud profiles, for the period when DARDAR is available, by more than six orders of magnitude and moreover, IceCloudNet is able to produce vertical cloud profiles beyond the lifetime of the recently ended satellite missions underlying DARDAR.
Kai Jeggle, David Neubauer, Gustau Camps-Valls, Ulrike Lohmann
Cirrus clouds are key modulators of Earth's climate. Their dependencies on meteorological and aerosol conditions are among the largest uncertainties in global climate models. This work uses three years of satellite and reanalysis data to study the link between cirrus drivers and cloud properties. We use a gradient-boosted machine learning model and a Long Short-Term Memory (LSTM) network with an attention layer to predict the ice water content and ice crystal number concentration. The models show that meteorological and aerosol conditions can predict cirrus properties with $R^2 = 0.49$. Feature attributions are calculated with SHapley Additive exPlanations (SHAP) to quantify the link between meteorological and aerosol conditions and cirrus properties. For instance, the minimum concentration of supermicron-sized dust particles required to cause a decrease in ice crystal number concentration predictions is $2 \times 10^{-4}$ mg m\textsuperscript{-3}. The last 15 hours before the observation predict all cirrus properties.
Kai Jeggle, Mikolaj Czerkawski, Federico Serva, Bertrand Le Saux, David Neubauer, Ulrike Lohmann
Clouds containing ice particles play a crucial role in the climate system. Yet they remain a source of great uncertainty in climate models and future climate projections. In this work, we create a new observational constraint of regime-dependent ice microphysical properties at the spatio-temporal coverage of geostationary satellite instruments and the quality of active satellite retrievals. We achieve this by training a convolutional neural network on three years of SEVIRI and DARDAR data sets. This work will enable novel research to improve ice cloud process understanding and hence, reduce uncertainties in a changing climate and help assess geoengineering methods for cirrus clouds.
Emilie Fons, Isabel L. McCoy, Tom Beucler, David Neubauer, Ulrike Lohmann
Biomass burning aerosols (BBAs) from Southern Africa seasonally overlie the semi-permanent South-East Atlantic (SEA) stratocumulus deck, impacting the region's energy budget through complex aerosol-cloud-radiation-meteorology interactions. Climate model intercomparison initiatives, like the Aerosol Comparisons between Observations and Models (AeroCom), have highlighted the large inter-model variability for BBA radiative effects, especially over the SEA, due to parameterization of emission modeling and smoke properties. Observational constraints are needed to reduce these uncertainties, but correlative observational studies are typically affected by confounding meteorological influences. We propose a physically informed statistical approach, based on causal graphs applied to satellite observations, to disentangle BBA influences on shortwave radiation over the SEA and identify the main sources of statistical biases plaguing observational studies. We find that, during the fire season, BBAs cause a regional shortwave cooling of -2.5 W m$^{-2}$, which can be decomposed into equal contributions from three physical pathways: aerosol-radiation interactions (ARI), adjustments to ARI, and aerosol-cloud interactions (ACI). We also perform ablation experiments with graph variants to investigate the main sources of confounding - like large-scale winds, humidity-biased retrievals or spatial aggregation of data - and show that they result in biased radiative effect estimates (between -50 $\%$ and +15 $\%$). Once free of such biases, our derived causal estimates of smoke radiative effects can be used as observational constraints to improve climate models.