Many-spin interactions and spin excitations in Mn 12
/ Authors
/ Abstract
In this work, the many-spin interactions taking place in ${\mathrm{Mn}}_{12}$ large-spin clusters are extensively studied using the 8-spin model Hamiltonian, for which we determine the possible parameters based on experimental data. Account of the many-spin excitations satisfactorily explains positions of the neutron scattering peaks, results of EPR measurements, and the temperature dependence of magnetic susceptibility. In particular, strong Dzyaloshinsky-Morya interactions are found to be important for description of neutron scattering data.
Journal: Physical Review B