Quantum phase transitions of a square-lattice Heisenberg antiferromagnet with two kinds of nearest-neighbor bonds: A high-order coupled-cluster treatment

We study the zero-temperature phase diagram and the low-lying excitations of a square-lattice spin-half Heisenberg antiferromagnet with two types of regularly distributed nearest-neighbor exchange bonds [J>0 (antiferromagnetic) and -infinity 0. For frustrating ferromagnetic couplings J'<0 we find indications that quantum fluctuations favor a first-order phase transition from the Neel order to a quantum helical state, by contrast with the corresponding second-order transition in the corresponding classical model. The results are compared to those of exact diagonalizations of finite systems (up to 32 sites) and those of spin-wave and variational calculations. The CCM results agree well with the exact diagonalization data over the whole range of the parameters. The special case of J'=0, which is equivalent to the honeycomb lattice, is treated more closely.