Room-temperature continuous-wave pumped exciton polariton condensation in a perovskite microcavity
/ Authors
Jiepeng Song, Sanjib Ghosh, Xinyi Deng, Chun Li, Qiuyu Shang, Xinfeng Liu, Yubin Wang, Xiaoyue Gao, Wenkai Yang, Xianjin Wang
and 6 more authors
Qing Zhao, Kebin Shi, Peng Gao, Guichuan Xing, Qihua Xiong, Qing Zhang
/ Abstract
Microcavity exciton polaritons (polaritons) as part-light part-matter quasiparticles garner considerable attention for Bose-Einstein condensation at elevated temperatures. Recently, halide perovskites have emerged as promising room-temperature polaritonic platforms because of their large exciton binding energies and superior optical properties. However, currently, inducing room-temperature nonequilibrium polariton condensation in perovskite microcavities requires optical pulsed excitations with high excitation densities. Here, we demonstrate continuous-wave optically pumped polariton condensation with an exceptionally low threshold of ~0.53 W cm−2 and a narrow linewidth of ~0.5 meV. Polariton condensation is unambiguously demonstrated by characterizing the nonlinear behavior and coherence properties. We also unveil the trapping potential landscape strategy to facilitate polariton relaxation and accumulation. Our findings lay the foundation for the next-generation energy-efficient polaritonic devices operating at room temperature.
Journal: Science Advances