Total absorption $γ$-ray spectroscopy of the $β$ decays of $^{96\text{gs,m}}$Y
nucl-ex
/ Authors
V. Guadilla, L. Le Meur, M. Fallot, J. A. Briz, M. Estienne, L. Giot, A. Porta, A. Cucoanes, T. Shiba, A. -A. Zakari-Issoufou
and 35 more authors
A. Algora, J. L. Tain, J. Agramunt, D. Jordan, M. Monserrate, A. Montaner-Pizá, E. Nácher, S. E. A. Orrigo, B. Rubio, E. Valencia, J. Äystö, T. Eronen, D. Gorelov, J. Hakala, A. Jokinen, A. Kankainen, V. Kolhinen, J. Koponen, I. Moore, H. Penttilä, I. Pohjalainen, J. Reinikainen, M. Reponen, S. Rinta-Antila
/ Abstract
The $β$ decays of the ground state (gs) and isomeric state (m) of $^{96}$Y have been studied with the total absorption $γ$-ray spectroscopy technique at the Ion Guide Isotope Separator On-Line facility. The separation of the 8$^{+}$ isomeric state from the 0$^{-}$ ground state was achieved thanks to the purification capabilities of the JYFLTRAP double Penning trap system. The $β$-intensity distributions of both decays have been independently determined. In the analyses the de-excitation of the 1581.6 keV level in $^{96}$Zr, in which conversion electron emission competes with pair production, has been carefully considered and found to have significant impact on the $β$-detector efficiency, influencing the $β$-intensity distribution obtained. Our results for $^{96\text{gs}}$Y (0$^+$) confirm the large ground state to ground state $β$-intensity probability, although a slightly larger value than reported in previous studies was obtained, amounting to $96.6_{-2.1}^{+0.3}\%$ of the total $β$ intensity. Given that the decay of $^{96\text{gs}}$Y is the second most important contributor to the reactor antineutrino spectrum between 5 and 7 MeV, the impact of the present results on reactor antineutrino summation calculations has been evaluated. In the decay of $^{96\text{m}}$Y (8$^{+}$), previously undetected $β$ intensity in transitions to states above 6 MeV has been observed. This shows the importance of total absorption $γ$-ray spectroscopy measurements of $β$ decays with highly fragmented de-excitation patterns. $^{96\text{m}}$Y (8$^{+}$) is a major contributor to reactor decay heat in uranium-plutonium and thorium-uranium fuels around 10 s after fission pulses, and the newly measured average $β$ and $γ$ energies differ significantly from the previous values in evaluated databases (...)