Isotropic Pauli-limited superconductivity in the infinite-layer nickelate Nd0.775Sr0.225NiO2

The recent observation of superconductivity in thin-film infinite-layer nickelates 1 – 3 offers a different angle from which to investigate superconductivity in layered oxides 4 . A wide range of candidate models have been proposed 5 – 10 , which emphasize single- or multi-orbital electronic structure, Kondo or Hund’s coupling and analogies to cuprates. Further experimental characterization of the superconducting state is needed to develop a full understanding of the nickelates. Here we use magnetotransport measurements to probe the superconducting anisotropy in Nd 0.775 Sr 0.225 NiO 2 . We find that the upper critical field is surprisingly isotropic at low temperatures despite the layered crystal structure. In a magnetic field, the superconductivity is strongly Pauli-limited, such that the paramagnetic effect dominates over orbital de-pairing. Underlying this isotropic response is a substantial anisotropy in the superconducting coherence length, which is at least four times longer in-plane than out-of-plane. A prominent low-temperature upturn in the upper critical field indicates the presence of an unconventional ground state. Measurements of a superconducting infinite-layer nickelate show that its upper critical field is largely isotropic despite its quasi-two-dimensional structure. This indicates that, unusually for layered oxides, the superconductivity is Pauli-limited.