Neutron Spin Resonance in a Quasi-Two-Dimensional Iron-Based Superconductor.

The neutron spin resonance is generally regarded as a key to understanding the magnetically mediated Cooper pairing in unconventional superconductors. Here, we report an inelastic neutron scattering study on the low-energy spin excitations in a quasi-two-dimensional iron-based superconductor KCa_{2}Fe_{4}As_{4}F_{2}. We have discovered a two-dimensional spin resonant mode with downward dispersions, a behavior closely resembling the low branch of the hourglass-type spin resonance in cuprates. While the resonant intensity is predominant by two broad incommensurate peaks near Q=(0.5,0.5) with a sharp energy peak at E_{R}=16 meV, the overall energy dispersion of the mode exceeds the measured maximum total gap Δ_{tot}=|Δ_{k}|+|Δ_{k+Q}|. These results deeply challenge the conventional understanding of the resonance modes as magnetic excitons regardless of underlining pairing symmetry schemes, and it also points out that when the iron-based superconductivity becomes very quasi-two-dimensional, the electronic behaviors are similar to those in cuprates.