Magnetic Excitations of the Classical Spin Liquid MgCr_{2}O_{4}.
/ Authors
X. Bai, J. Paddison, J. Paddison, E. Kapit, E. Kapit, S. Koohpayeh, Jiajia Wen, Siân E. Dutton, A. Savici, A. I. Kolesnikov
and 6 more authors
G. Granroth, C. Broholm, C. Broholm, J. Chalker, M. Mourigal, M. Mourigal
/ Abstract
We report a comprehensive inelastic neutron-scattering study of the frustrated pyrochlore antiferromagnet MgCr_{2}O_{4} in its cooperative paramagnetic regime. Theoretical modeling yields a microscopic Heisenberg model with exchange interactions up to third-nearest neighbors, which quantitatively explains all of the details of the dynamic magnetic response. Our work demonstrates that the magnetic excitations in paramagnetic MgCr_{2}O_{4} are faithfully represented in the entire Brillouin zone by a theory of magnons propagating in a highly correlated paramagnetic background. Our results also suggest that MgCr_{2}O_{4} is proximate to a spiral spin-liquid phase distinct from the Coulomb phase, which has implications for the magnetostructural phase transition in MgCr_{2}O_{4}.
Journal: Physical review letters