Geometric phase magnetometry using a solid-state spin

Magnetometry is a powerful technique for the non-invasive study of biological and physical systems. A key challenge lies in the simultaneous optimization of magnetic field sensitivity and maximum field range. In interferometry-based magnetometry, a quantum two-level system acquires a dynamic phase in response to an applied magnetic field. However, due to the 2π periodicity of the phase, increasing the coherent interrogation time to improve sensitivity results in reduced field range. Here we introduce a route towards both large magnetic field range and high sensitivity via measurements of the geometric phase acquired by a quantum two-level system. We experimentally demonstrate geometric-phase magnetometry using the optically addressable electronic spin associated with the nitrogen vacancy (NV) color center in diamond. Our approach enables unwrapping of the 2π phase ambiguity, decoupling of magnetic field range from sensitivity, and enhancement of the field range by about 400 times. We also find additional improvement in sensitivity in the nonadiabatic regime, and study how geometric-phase decoherence depends on adiabaticity. Our results show that the geometric phase can be a versatile tool for quantum sensing applications.