Strong Exciton-Photon Coupling and lasing behavior in All-Inorganic CsPbBr3 Micro/nanowire Fabry-Perot cavity

Macroscopic spontaneous coherence of exciton-polariton in semiconductor cavity is one important research field in condensed matter physics. All-inorganic micro/nanowire Fabry-Pérot cavity with excellent optical performance makes it possible to realize strong coupling and lasing of exciton-photon at room temperature. In this work, we demonstrated strong coupling of exciton-photon and polariton lasing in CsPbBr3 micro/nanowires synthesized by CVD method. By exploring spatial resolved PL spectra of CsPbBr3 cavity, we observed mode volume dependent coupling strength , as well as significant increase in group index. Moreover, low threshold polariton lasing was achieved at room temperature within strong coupling regime; the polariton characteristic is confirmed by comparing lasing spectra with waveguided output spectra and the dramatically reduced lasing threshold. Our present results provide new avenues to achieve high coupling strengths potentially enabling application of exciting phenomena such as Bose-Einstein condensation of polaritons, efficient light-emitting diodes and lasers.