Ultrafast THz Field Control of Electronic and Structural Interactions in Vanadium Dioxide
cond-mat.str-el
/ Authors
A. X. Gray, M. C. Hoffmann, J. Jeong, N. P. Aetukuri, D. Zhu, H. Y. Hwang, N. C. Brandt, H. Wen, A. J. Sternbach, S. Bonetti
and 27 more authors
A. H. Reid, R. Kukreja, C. Graves, T. Wang, P. Granitzka, Z. Chen, D. J. Higley, T. Chase, E. Jal, E. Abreu, M. K. Liu, T. -C. Weng, D. Sokaras, D. Nordlund, M. Chollet, H. Lemke, J. Glownia, M. Trigo, Y. Zhu, H. Ohldag, J. W. Freeland, M. G. Samant, J. Berakdar, R. D. Averitt
/ Abstract
Vanadium dioxide, an archetypal correlated-electron material, undergoes an insulator-metal transition near room temperature that exhibits electron-correlation-driven and structurally-driven physics. Using ultrafast optical spectroscopy and x-ray scattering we show that these processes can be disentangled in the time domain. Specifically, following intense sub-picosecond electric-field excitation, a partial collapse of the insulating gap occurs within the first ps. Subsequently, this electronic reconfiguration initiates a change in lattice symmetry taking place on a slower timescale. We identify the kinetic energy increase of electrons tunneling in the strong electric field as the driving force, illustrating a novel method to control electronic interactions in correlated materials on an ultrafast timescale.