Ground-state phase diagram of the spin-(1)/(2) square-lattice J 1 -J 2 model with plaquette structure

Using the coupled-cluster method for high orders of approximation and Lanczos exact diagonalization we study the ground-state phase diagram of a quantum spin-$\frac{1}{2}$ ${J}_{1}$-${J}_{2}$ model on the square lattice with plaquette structure. We consider antiferromagnetic (${J}_{1}g0$) as well as ferromagnetic (${J}_{1}l0$) nearest-neighbor interactions together with frustrating antiferromagnetic next-nearest-neighbor interaction ${J}_{2}g0$. The strength of interplaquette interaction $\ensuremath{\lambda}$ varies between $\ensuremath{\lambda}=1$ (which corresponds to the uniform ${J}_{1}$-${J}_{2}$ model) and $\ensuremath{\lambda}=0$ (which corresponds to isolated frustrated 4-spin plaquettes). While on the classical level ($s\ensuremath{\rightarrow}\ensuremath{\infty}$) both versions of models (i.e., with ferro- and antiferromagnetic ${J}_{1}$) exhibit the same ground-state behavior, the ground-state phase diagram differs basically for the quantum case $s=1/2$. For the antiferromagnetic case (${J}_{1}g0$) N\'eel antiferromagnetic long-range order at small ${J}_{2}/{J}_{1}$ and $\ensuremath{\lambda}\ensuremath{\gtrsim}0.47$ as well as collinear striped antiferromagnetic long-range order at large ${J}_{2}/{J}_{1}$ and $\ensuremath{\lambda}\ensuremath{\gtrsim}0.30$ appear which correspond to their classical counterparts. Both semiclassical magnetic phases are separated by a nonmagnetic quantum paramagnetic phase. The parameter region, where this nonmagnetic phase exists, increases with decreasing $\ensuremath{\lambda}$. For the ferromagnetic case (${J}_{1}l0$) we have the trivial ferromagnetic ground state at small ${J}_{2}/|{J}_{1}|$. By increasing ${J}_{2}$ this classical phase gives way for a semiclassical plaquette phase, where the plaquette block spins of length $s=2$ are antiferromagnetically long-range ordered. Further increasing of ${J}_{2}$ then yields collinear striped antiferromagnetic long-range order for $\ensuremath{\lambda}\ensuremath{\gtrsim}0.38$, but a nonmagnetic quantum paramagnetic phase $\ensuremath{\lambda}\ensuremath{\lesssim}0.38$.